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This research investigated the motivations of volunteers for World Expo 2010 Shanghai China and examined the relationships between their motivations and job satisfaction. An on-site survey was conducted with volunteers working at the event. An exploratory factor analysis delineated five underlying dimensions: Values, Learning, Career, Social, and Civic Responsibility. The results of this study indicate that these dimensions have a positive effect on volunteers’ job satisfaction. The findings of this study suggest that the measurement scale for volunteers’ motivations adapted for the World Expo 2010 Shanghai could be reliable when examining the motivations of volunteers at mega-events.